Biomedical Engineering Reference
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pulse width long enough to capture several Rabi oscillations of the excitonic level
populations. When, e B ( T ) ,
, the resulting Hamiltonian basis contains
a total of 14 neutral exciton states. This corresponds to: the vacuum 0 00 X ; a pair of
monoexcitons 1 10 X
h B ( T ) = {
0
,
1
,
2
}
01
01 X ; a pair of spatially indirect monoexcitons, 1 01 X
01
,
,
10 X ; direct
biexciton states 2 20 X
02
02 X ; indirect biexciton states 2 02 X
02
,
,
20 X ; a delocalized biexciton
11
11 X and a remaining set of trion-like states, 0 11 X
20
11
11
20 X .
Up to single occupancy of holes and electrons, e B ( T ) ,
,
11 X
,
02 X
,
, the per-
turbed Hamiltonian corresponding to the monoexciton manifold in ( 10.8 ), is
given by
h B ( T ) = {
0
,
1
}
H tot
=
H D
+
H tun
+
H V F +
H opt
.
(10.10)
The Hamiltonian in ( 10.10 ) includes the diagonal contribution of ( 10.8 )plusthe
vacuum state
, the tunneling matrix elements of electrons and holes, H tun ,
the resonant energy transfer interaction, V F , and the laser excitation or optical
perturbation, H opt . Explicitly,
|
0
| + i
H D = |
0
0
E i |
i
i
|
t e
c
t h
c
01
01 X
01
10 X
01
01 X
01
10 X
H tun =
|
| +
H
.
+
|
| +
H
.
V F
c
01
01 X
10
10 X
H V F =
|
| +
H
.
H opt = Ω T e i ω t
+ Ω B e i ω t
01
01 X
e i ω t
01
01 X
10
10 X
e i ω t
10
10 X
|
0
| +
|
0
|
|
0
| +
|
0
|
.
(10.11)
In the model, only spatially direct monoexcitons are coupled to the radiation
field by
0 01 X
1 10 X
, for QD(T) and
QD(B), respectively. On the other hand, the spatially indirect excitons have typically
a much weaker oscillator strength; its inclusion in the model is straightforward
but will be ignored in what follows. Here,
Ω T (
t
)=
0
| μ T ·
E
(
t
) |
and
Ω B (
t
)=
0
| μ B ·
E
(
t
) |
μ i are the interband transition dipole
moments and E
is the electric field component of the radiation pulse amplitude.
In order to simplify the equation of motion, we have performed the rotating
wave approximation (RWA) and a unitary transformation that removes the time-
dependent fast oscillatory terms of the matter-radiation interaction [ 24 ]. The latter
approximation is carried out by the following transformation,
(
t
)
ih ∂Λ
H
H
= Λ
Λ +
Λ
t
Λ = k
e i ξ k t
|
k
k
|,
(10.12)
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