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chain that shows reversible dehydration-rehydration with retention of single
crystallinity. Other MMX chains with binary countercations also shows reversible
dehydration-rehydration
except
the MMX chains
containing
longer
alkyldiammonium ion (B 2+
NC 5 N 2+ ,NC 2 OC 2 N 2+ ). Various spectroscopic
analyses indicated that the electronic state of K 2 (NC 3 N)[Pt 2 (pop) 4 I] is CDW
state but is close to the border of CDW and AV state because the band gap is
very small and the solitons are excited at room temperature. MMX chains with
binary countercations are also the first examples that show vapor-induced revers-
ible switching of electrical conductivity in MMX chains. The robustness of the
complexes becomes weaker as the length of B 2+
¼
of the complexes becomes
longer.
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