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Cl
OMe
F
Br
(Ph 3 P) 4 Pd
+
Cl
Cl
OMe
DME/H 2 O
NaOH, 80°C
Cl
B(OH) 2
F
NH 2
20 kg scale
O Cl
Cl
5-HT 2C receptor antagonist
F
Scheme 3.4 Wyeth's synthesis of a 5-HT 2C receptor antagonist using a chemoselec-
tive Suzuki-Miyaura coupling.
I
N
(Ph 3 P) 4 Pd
THF, rt
+
NN
N
l
N
N
Cl
Cl
Scheme 3.5 Chemoselective Negishi coupling of an aryl iodide.
compared with the use of more advanced Pd precatalysts with higher
reactivities.
Gontcharov et al. at Wyeth Research disclosed a process to make a 5-HT 2C
receptor antagonist in which the first step consisted of a (Ph 3 P) 4 Pd-catalyzed
Suzuki-Miyaura coupling reaction carried out on a 20 kg scale
(Scheme 3.4). 30 In this case, the chemoselective coupling of a chloride-
containing aryl bromide was achieved. This may have proved to be chal-
lenging in terms of selectivity while using a more active precatalyst.
In 2007, a Negishi cross-coupling between the in situ-prepared 2-pyr-
idylzinc chloride and 5-iodo-2-chloropyrimidine catalyzed by (Ph 3 P) 4 Pd af-
forded the product in a single step on a kilogram scale (Scheme 3.5). 31 This
chemoselective coupling of a chloride-containing aryl iodide is particularly
noteworthy, as the chloride is in the inherently most reactive position for a
standard S N Ar reaction.
3.5 L 2 Pd(0) Complexes
The use of triarylphosphines such as Ph 3 P as ligands limits the scope of the
aryl halide substrate to aryl iodides or activated aryl bromides. Since aryl
chlorides would be desirable substrates from a cost point of view as they are
industrial feedstocks, substantial research efforts have been focused on
overcoming this limitation. The use of trialkyl- and dialkyl-based phosphine
ligands came as a breakthrough in this area (see Chapter 2 for details), al-
though some of these ligands are air sensitive or even pyrophoric in nature,
posing safety concerns especially during scale-up. Such risks are avoided
by using preformed Pd catalysts of these ligands, where the complexes
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