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Acknowledgments We owe great thanks to the crew and scientific party on board the R/V
Hakuho-maru during cruise KH-98-1. An early version of this manuscript was reviewed by and
discussed with Drs. Yumul, G.P. Jr., Daniel Curewitz, Hidetsugu Taniguchi and Yasuhiko Ohara,
to whom we are grateful. We appropriate Shinji Kanayama for his help with the XRF sample
preparation.
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